Microwave-Assisted Synthesis of Highly-Crumpled, Few-Layered Graphene and Nitrogen-Doped Graphene for Use as High-Performance Electrodes in Capacitive Deionization

Amiri, A. and Ahmadi, G. and Shanbedi, M. and Savari, M. and Kazi, S.N. and Chew, B.T. (2015) Microwave-Assisted Synthesis of Highly-Crumpled, Few-Layered Graphene and Nitrogen-Doped Graphene for Use as High-Performance Electrodes in Capacitive Deionization. Scientific Reports, 5. ISSN 2045-2322,

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Official URL: DOI: 10.1038/srep17503

Abstract

Capacitive deionization (CDI) is a promising procedure for removing various charged ionic species from brackish water. The performance of graphene-based material in capacitive deionization is lower than the expectation of the industry, so highly-crumpled, few-layered graphene (HCG) and highly-crumpled nitrogen-doped graphene (HCNDG) with high surface area have been introduced as promising candidates for CDI electrodes. Thus, HCG and HCNDG were prepared by exfoliation of graphite in the presence of liquid-phase, microwave-assisted methods. An industrially-scalable, cost-effective, and simple approach was employed to synthesize HCG and HCNDG, resulting in few-layered graphene and nitrogen-doped graphene with large specific surface area. Then, HCG and HCNDG were utilized for manufacturing a new class of carbon nanostructure-based electrodes for use in large-scale CDI equipment. The electrosorption results indicated that both the HCG and HCNDG have fairly large specific surface areas, indicating their huge potential for capacitive deionization applications.

Item Type: Article
Funders: UNSPECIFIED
Uncontrolled Keywords: Oxygen reduction reaction; Water desalination; Carbon composites; Facile synthesis; Metal nitride;Oxide; Nanoparticles; Nanosheets; Membrane; Sponge
Subjects: Q Science > Q Science (General)
T Technology > T Technology (General)
Depositing User: Mrs. Siti Mawarni Salim
Date Deposited: 11 Aug 2016 03:01
Last Modified: 27 Aug 2019 07:45
URI: http://eprints.um.edu.my/id/eprint/16228

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