Contributions of symmetric metal contacts on liquid exfoliation 2D-MoS2 flakes based MSM photodetector by spray pyrolysis: A CVD-free technique

Ripain, A. H. Abdullah and Zulkifli, N. A. A. and Tan, C. L. and Abd Majid, Wan Haliza and Zakaria, Rozalina (2022) Contributions of symmetric metal contacts on liquid exfoliation 2D-MoS2 flakes based MSM photodetector by spray pyrolysis: A CVD-free technique. Optical and Quantum Electronics, 54 (12). ISSN 0306-8919, DOI https://doi.org/10.1007/s11082-022-04253-y.

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Abstract

Molybdenum disulphide (MoS2), is a typical layered of transition metal dichalcogenides which has been considered as a strong candidate in many optoelectronic devices due to its layer dependent bandgap and tunability properties. We reported a high yield synthesis of MoS2 flakes prepared using mixed solvent exfoliation followed by feasible and cost-effective spray pyrolysis deposition, in other words; chemical vapor deposition (CVD) free technique. The photodetector based on MoS2 flakes is fabricated using electron beam evaporation (e-beam) with symmetrical metals of Au and Ag contacts. The measurements were carried out under 632 nm illumination at power intensity ranging from 0.792 to 2.537 mW/cm(2). The symmetrical of Au-MoS2/Si-based PD showed the highest photoresponsivity of 128.0 mA/W and specific detectivity of 1.32 x 10(10) Jones. This work demonstrates fecund synthesis of good quality MoS2 flakes and the significance of metal choice in the photodetector as well as Schottky barrier height tuning which a good indicator for enhancing the device performance.

Item Type: Article
Funders: SATU grant under University Malaya (Grant No: STU048-2021)
Uncontrolled Keywords: MoS2-TMDC; Spray-pyrolysis; Metal-semiconductor-metal (MSM); Photodetector
Subjects: Q Science > QC Physics
Divisions: Faculty of Science > Department of Physics
Deputy Vice Chancellor (Research & Innovation) Office > Photonics Research Centre
Depositing User: Ms. Juhaida Abd Rahim
Date Deposited: 14 Nov 2023 07:23
Last Modified: 14 Nov 2023 07:23
URI: http://eprints.um.edu.my/id/eprint/40711

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