Cellulose nanocomposite tough hydrogels: synergistic self-healing, adhesive and strain-sensitive properties

Badawi, Mohammed Nujud and Agrawal, Namrata and Kumar, Yogesh and Khan, Mujeeb and Hatshan, Mohammad Rafe and Alayyaf, Abdulmajeed Abdullah and Adil, Syed Farooq (2024) Cellulose nanocomposite tough hydrogels: synergistic self-healing, adhesive and strain-sensitive properties. Polymer International, 73 (9). pp. 748-760. ISSN 0959-8103, DOI https://doi.org/10.1002/pi.6644.

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Official URL: https://doi.org/10.1002/pi.6644

Abstract

Recent advancements are notable in electrically conductive hydrogels emulating human skin functions. However, a significant challenge remains: crafting a single conductive gel that integrates self-healing, robust mechanical strength, and excellent electrical traits. Our innovation lies in a strong, lightweight, curable gel achieved through multiple coordination bonds between cellulose crystals and acid-treated multi-walled carbon nanotubes (MWCNTs) in a polymer network. Embedded MWCNTs act as dynamic bridges within a porous structure, giving exceptional mechanical performance. Reversible coordination interactions confer remarkable recovery and reliable mechanical and electrical self-healing. Additionally, these ionic gels function as adaptable stress sensors, detecting significant movements like finger and joint motions. This work introduces MWCNT-incorporated nanomaterials with good stretchability, high ion conductivity, remarkable self-healing nature, and good stress sensitivity. Such proteins hold promise for electronic sensors, wearable devices, and healthcare monitoring, unveiling a path to diverse applications. Our study addresses challenges and unlocks possibilities for materials that can adapt, withstand, and sense in innovative ways. (c) 2024 Society of Chemical Industry. Strong, lightweight, curable gel through multiple coordination bonds between cellulose crystals and acid-treated multi-walled carbon nanotubes (MWCNTs) in a polymer network. Embedded MWCNTs act as dynamic bridges within a porous structure, giving exceptional mechanical performance. image

Item Type: Article
Funders: Researchers supporting project, King Saud University, Riyadh, Saudi Arabia (RSP2024R222), King Saud University
Uncontrolled Keywords: conductive gels; highly ionic conducting; hydrogen bond; self-healing materials
Subjects: Q Science > Q Science (General)
Q Science > QC Physics
Divisions: Faculty of Science > Department of Physics
Depositing User: Ms. Juhaida Abd Rahim
Date Deposited: 15 Jan 2025 07:19
Last Modified: 15 Jan 2025 07:19
URI: http://eprints.um.edu.my/id/eprint/46920

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