Polycaprolactone/starch composite: Fabrication, structure, properties, and applications

Ghavimi, S.A.A. and Ebrahimzadeh, M.H. and Solati-Hashjin, M. and Abu Osman, Noor Azuan (2015) Polycaprolactone/starch composite: Fabrication, structure, properties, and applications. Journal of Biomedical Materials Research Part A, 103 (7). pp. 2482-2498. ISSN 1549-3296, DOI https://doi.org/10.1002/jbm.a.35371.

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Abstract

Interests in the use of biodegradable polymers as biomaterials have grown. Among the different polymeric composites currently available, the blend of starch and polycaprolactone (PCL) has received the most attention since the 1980s. Novamont is the first company that manufactured a PCL/starch (SPCL) composite under the trademark Mater-Bi (R). The properties of PCL (a synthetic, hydrophobic, flexible, expensive polymer with a low degradation rate) and starch (a natural, hydrophilic, stiff, abundant polymer with a high degradation rate) blends are interesting because of the composite components have completely different structures and characteristics. PCL can adjust humidity sensitivity of starch as a biomaterial; while starch can enhance the low biodegradation rate of PCL. Thus, by appropriate blending, SPCL can overcome important limitations of both PCL and starch components and promote controllable behavior in terms of mechanical properties and degradation which make it suitable for many biomedical applications. This article reviewed the different fabrication and modification methods of the SPCL composite; different properties such as structural, physical, and chemical as well as degradation behavior; and different applications as biomaterials. (c) 2014 Wiley Periodicals, Inc. J Biomed Mater Res Part A: 103: 2482-2498, 2015.

Item Type:	Article
Funders:	High Impact Research Grant from the University of Malaya UM.C/HIR/MOHE/ENG/10 D000010-16001
Additional Information:	ISI Document Delivery No.: CJ1LZ Times Cited: 0 Cited Reference Count: 206 Cited References: Abbasi Z, 2014, INT J NANODIMENSION, V5, P549 Ajili SH, 2009, ACTA BIOMATER, V5, P1519, DOI 10.1016/j.actbio.2008.12.014 Ali SFA, 2014, J POLYM ENVIRON, V22, P359, DOI 10.1007/s10924-014-0675-6 AliAkbari Ghavimi S, 2012, J TISSUE ENG REGE S1, P12 Aliakbari Ghavimi S., 2012, MODARES J MED SCI PA, V15, P37 Alix S, 2013, EUR POLYM J, V49, P1234, DOI 10.1016/j.eurpolymj.2013.03.016 Alves CM, 2007, BIOMATERIALS, V28, P307, DOI 10.1016/j.biomaterials.2006.09.010 Arvanitoyannis I, 1997, STARCH-STARKE, V49, P306, DOI 10.1002/star.19970490712 Avella M, 2000, POLYMER, V41, P3875, DOI 10.1016/S0032-3861(99)00663-1 Averous L, 2001, POLYM ENG SCI, V41, P727, DOI 10.1002/pen.10768 Averous L, 2004, J MACROMOL SCI-POL R, VC44, P231, DOI 10.1081/mc-200029326 Averous L, 2000, POLYMER, V41, P4157, DOI 10.1016/S0032-3861(99)00636-9 Azevedo HS, 2003, BIOMACROMOLECULES, V4, P1703, DOI 10.1021/bm0300397 Azevedo HS, 2009, ACTA BIOMATER, V5, P3021, DOI 10.1016/j.actbio.2009.04.039 Balmayor ER, 2009, ACTA BIOMATER, V5, P1035, DOI 10.1016/j.actbio.2008.11.006 Bastioli C, 1998, MACROMOLECULAR S BASTIOLI C, 1995, J ENVIRON POLYM DEGR, V3, P81, DOI 10.1007/BF02067484 Belard L, 2009, POLYM ENG SCI, V49, P1177, DOI 10.1002/pen.21342 Beneke CE, 2009, MOLECULES, V14, P2602, DOI 10.3390/molecules14072602 Cai J, 2014, CARBOHYD POLYM, V102, P746, DOI 10.1016/j.carbpol.2013.10.095 Campos A, 2012, J REINF PLAST COMP, V31, P573, DOI 10.1177/0731684412441092 Campos A, 2012, POLYM DEGRAD STABIL, V97, P1948, DOI 10.1016/j.polymdegradstab.2011.11.010 Carmona VB, 2014, J THERM ANAL CALORIM, V115, P153, DOI 10.1007/s10973-013-3259-0 Carvalho PP, 2014, J BIOMED MATER RES A, V102, P3102, DOI 10.1002/jbm.a.34983 Chandra R, 1998, PROG POLYM SCI, V23, P1273, DOI 10.1016/S0079-6700(97)00039-7 Chang PR, 2009, J APPL POLYM SCI, V113, P2973, DOI 10.1002/app.30369 Chen L, 2005, CARBOHYD POLYM, V60, P103, DOI 10.1016/j.carbpol.2004.11.028 Chivrac F, 2009, MAT SCI ENG R, V67, P1, DOI 10.1016/j.mser.2009.09.002 Cho HS, 2011, WASTE MANAGE, V31, P475, DOI 10.1016/j.wasman.2010.10.029 Choi EJ, 1999, J POLYM SCI POL PHYS, V37, P2430, DOI 10.1002/(SICI)1099-0488(19990901)37:17<2430::AID-POLB14>3.0.CO;2-4 Choi EJ, 1999, MACROMOLECULES, V32, P7402, DOI 10.1021/ma981453f Costa SA, 2004, J MATER SCI-MATER M, V15, P335, DOI 10.1023/B:JMSM.0000021098.75103.3a Cyras VP, 2002, J THERMOPLAST COMPOS, V15, P253, DOI 10.1106/089270502021454, 10.1006/089270502021454 Cyras VP, 2001, POLYM ENG SCI, V41, P1521, DOI 10.1002/pen.10851 da Silva M. 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Solati-Hashjin, Mehran Abu Osman, Noor Azuan Engineering, Faculty /I-7935-2015 Engineering, Faculty /0000-0002-4848-7052 High Impact Research Grant from the University of Malaya UM.C/HIR/MOHE/ENG/10 D000010-16001 Contract grant sponsor: High Impact Research Grant from the University of Malaya; contract grant number: UM.C/HIR/MOHE/ENG/10 D000010-16001 0 WILEY-BLACKWELL HOBOKEN J BIOMED MATER RES A
Uncontrolled Keywords:	Polycaprolactone, starch, polymeric composite, tissue engineering, degradation, POLY-EPSILON-CAPROLACTONE, TISSUE ENGINEERING APPLICATIONS, STARCH-BASED, BIOMATERIALS, RING-OPENING POLYMERIZATION, FIBER-MESH SCAFFOLDS, MARROW, STROMAL CELLS, DRUG-DELIVERY SYSTEMS, FOOD-PACKAGING APPLICATIONS, FLOW, PERFUSION BIOREACTOR, NATURAL ORIGIN SCAFFOLDS,
Subjects:	T Technology > T Technology (General) T Technology > TA Engineering (General). Civil engineering (General)
Divisions:	Faculty of Engineering
Depositing User:	Mr Jenal S
Date Deposited:	17 Mar 2016 01:25
Last Modified:	07 Feb 2019 07:41
URI:	http://eprints.um.edu.my/id/eprint/15715

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